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Create Document Library In Sharepoint. From the menu bar click on New and choose Document library. In the Document Template section under the Template.
Enter a name and description for the new document library in the dialogue box that appears and click Create. On the Account tab locate the synced library you wish to remove and click the Stop sync for that library. Enter a name for the new library.
On the File menu click Publish.
Also note that the Office files to be uploaded to the template libraries must be in a template format for example dotx for Word potx for PowerPoint and xltx for Excel. In the Enter the location of your SharePoint or InfoPath Forms Services. Select Form Webpart Default Edit Form. Multiple document libraries concept.